Search results for "nitric acid trihydrate"

showing 2 items of 2 documents

Nitric Acid Trihydrate (NAT) formation at low NAT supersaturation in Polar Stratospheric Clouds (PSCs)

2005

International audience; A PSC was detected on 6 February 2003 in the Arctic stratosphere by in-situ measurements onboard the high-altitude research aircraft Geophysica. Low number densities (~10-4cm-3) of small nitric acid (HNO3) containing particles (dTNAT, these NAT particles have the potential to grow further and to remove HNO3 from the stratosphere, thereby enhancing polar ozone loss. Interestingly, the NAT particles formed in less than a day at temperatures just slightly below TNAT (T>TNAT-3.1K). This unique measurement of PSC formation at extremely low NAT saturation ratios (SNAT?10) constrains current NAT nucleation theories. We suggest, that the NAT particles have formed heterogeneo…

Atmospheric Science010504 meteorology & atmospheric sciencesAnalytical chemistryNucleation010402 general chemistryAtmospheric sciences01 natural scienceslcsh:Chemistrychemistry.chemical_compoundNitric acidStratosphere0105 earth and related environmental sciences[SDU.OCEAN]Sciences of the Universe [physics]/Ocean AtmosphereSupersaturationChemistrylcsh:QC1-9990104 chemical sciencesThe arcticozonelcsh:QD1-99913. Climate actionNatpolar stratospheric cloud (PSC)PolarSaturation (chemistry)nitric acid trihydrate (NAT)lcsh:Physics
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Nitric acid trihydrate nucleation and denitrification in the Arctic stratosphere

2014

Abstract. Nitric acid trihydrate (NAT) particles in the polar stratosphere have been shown to be responsible for vertical redistribution of reactive nitrogen (NOy). Recent observations by Cloud–Aerosol Lidar with Orthogonal Polarization (CALIOP) aboard the CALIPSO satellite have been explained in terms of heterogeneous nucleation of NAT on foreign nuclei, revealing this to be an important formation pathway for the NAT particles. In state of the art global- or regional-scale models, heterogeneous NAT nucleation is currently simulated in a very coarse manner using a constant, saturation-independent nucleation rate. Here we present first simulations for the Arctic winter 2009/2010 applying a n…

Atmospheric ScienceDenitrification010504 meteorology & atmospheric sciencesForward scatterNucleationAtmospheric sciences01 natural sciences010309 opticslcsh:Chemistry0103 physical sciencesddc:550Life ScienceStratosphere0105 earth and related environmental sciencesSpectrometerozone holeChemistryAtmosphärische Spurenstoffelcsh:QC1-999Earth sciencesLidarnitric acid trihydratelcsh:QD1-99913. Climate actionPolarParticle sizelcsh:PhysicsArctic stratosphere
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